2025, №4

pp. 3-19

Co-Hydrolysis of GeCl4 and Pr(NO3)3 · 5H2O in an Aprotic Solvent — a Way to Create Aerogels with Target Luminescent Characteristics

2025, №4

сс. 3-19

Quote

O.M. Gajtko, S.V. Golodukhina, V.O. Veselova, D.A. Khvoshchevskaya, S.Yu. Kottsov, A.A. Sadovnikov, A.G. Son.

Key words: aerogel, germanium oxide, doping, praseodymium, co-gelation, luminescence

A straightforward method for creating crystalline GeO2: Pr3+ aerogels is introduced. By adapting an existing epoxide-induced synthesis process, we successfully performed cogelation of GeCl4 and Pr(NO3)3 · 5H2O. It was shown show that the concentration of the dopant ion in the aerogel increases in direct proportion to its initial share in the mixture, with a uniform distribution throughout the material. The dependence of the photoluminescence of GeO2: Pr3+ aerogels on the excitation wavelength is established. At high excitation energies, the luminescence is completely determined by the germanium oxide matrix, while when excited by green light, the characteristic orange-red emission bands of Pr3+ ions become the dominant.

doi:10.34984/SCFTP.2025.20.4.001